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【Dongdong Yan】
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Highly efficient emission and high-CRI warm white light-emitting diodes from ligand-modified CsPbBr
3
quantum dots
Download:547次
Dongdong Yan
1†
Shuangyi Zhao
1†
Yubo Zhang
2
Huaxin Wang
1
Zhigang Zang
1,*
Author Affiliations
Abstract
1
Key Laboratory of Optoelectronic Technology & Systems (Ministry of Education), Chongqing University, Chongqing 400044, China
2
Department of Physics, Southern University of Science and Technology, Shenzhen 518055, China
All-inorganic CsPbBr
3
perovskite quantum dots (QDs) have received great attention in white light emission because of their outstanding properties. However, their practical application is hindered by poor stability. Herein, we propose a simple strategy to synthesize excellent stability and efficient emission of CsPbBr
3
QDs by using 2-hexyldecanoic acid (DA) as a ligand to replace the regular oleic acid (OA) ligand. Thanks to the strong binding energy between DA ligand and QDs, the modified QDs not only show a high photoluminescence quantum yield (PLQY) of 96% but also exhibit high stability against ethanol and water. Thereby warm white light-emitting diodes (WLEDs) are constructed by combining ligand modified CsPbBr
3
QDs with red AgInZnS QDs on blue emitting InGaN chips, exhibiting a color rendering index of 93, a power efficiency of 64.8 lm/W, a CIE coordinate of (0.44, 0.42) and correlated color temperature value of 3018 K. In addition, WLEDs based on ligand modified CsPbBr
3
QDs also exhibit better thermal performance than that of WLEDs based on the regular CsPbBr
3
QDs. The combination of improved efficiency and better thermal stability with high color quality indicates that the modified CsPbBr
3
QDs are ideal for WLEDs application.
CsPbBr3 quantum dots
ligand modification
stability
efficiency
white light-emitting diodes
PDF全文
Full Text
Opto-Electronic Advances
2022, 5(1): 200075
Optical and Photonic Materials
Room temperature synthesis of stable silica-coated CsPbBr
3
quantum dots for amplified spontaneous emission
Download:782次
Qionghua Mo
1†
Tongchao Shi
2†
Wensi Cai
1
Shuangyi Zhao
1,*
[ ... ]
Zhigang Zang
1,5
Author Affiliations
Abstract
1
Key Laboratory of Optoelectronic Technology & Systems (Ministry of Education), Chongqing University, Chongqing 400044, China
2
State Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China
3
Hangzhou Institute for Advanced Study, University of Chinese Academy of Sciences, Hangzhou 310024, China
4
e-mail: dujuan@mail.siom.ac.cn
5
e-mail: zangzg@cqu.edu.cn
All-inorganic cesium lead bromide (
CsPbBr
3
) perovskite quantum dots (QDs) with excellent optical properties have been regarded as good gain materials for amplified spontaneous emission (ASE). However, the poor stability as the results of the high sensitivity to heat and moisture limits their further applications. Here, we report a facile one-pot approach to synthesize
CsPbBr
3
@
SiO
2
QDs at room temperature. Due to the effective defects passivation using
SiO
2
, as-prepared
CsPbBr
3
@
SiO
2
QDs present an enhanced photoluminescence quantum yield (PLQY) and chemical stability. The PLQY of
CsPbBr
3
@
SiO
2
QDs reaches 71.6% which is higher than 46% in pure
CsPbBr
3
QDs. The PL intensity of
CsPbBr
3
@
SiO
2
QDs maintains 84% while remaining 24% in pure
CsPbBr
3
after 80 min heating at 60°C. The ASE performance of the films is also studied under a two-photon-pumped laser. Compared with the films using pure
CsPbBr
3
QDs, those with as-prepared
CsPbBr
3
@
SiO
2
QDs exhibit a reduced threshold of ASE. The work suggests that room-temperature-synthesized
SiO
2
-coated perovskites QDs are promising candidates for laser devices.
PDF全文
Full Text
Photonics Research
2020, 8(10): 10001605
Optical and Photonic Materials
Ultrapure and highly efficient green light emitting devices based on ligand-modified CsPbBr
3
quantum dots
Download:782次
Dongdong Yan
Shuangyi Zhao
Huaxin Wang
Zhigang Zang
*
Author Affiliations
Abstract
Key Laboratory of Optoelectronic Technology & Systems (Ministry of Education), Chongqing University, Chongqing 400044, China
All inorganic
CsPbBr
3
perovskite quantum dots (QDs) have been recognized as promising optical materials to fabricate green light emission devices because of their excellent optical performance. However, regular
CsPbBr
3
QDs with an oleic acid (OA) ligand show poor stability, which limits their practical application. We replaced the OA ligand in
CsPbBr
3
QDs with a 2-hexyldecanoic acid (DA) ligand and, in the synthesis, found that the new material has better optical properties than regular
CsPbBr
3
QDs (
CsPbBr
3
-
OA
QDs). Due to the strong binding energy between the DA ligand and QDs, the ligand-modified
CsPbBr
3
QDs (
CsPbBr
3
-
DA
QDs) show a high photoluminescence quantum yield (PLQY) of 96%, while the PLQY of
CsPbBr
3
-
OA
QDs is 84%. Subsequently, the
CsPbBr
3
QDs coated on the blue light-emitting diode (LED) chips as green phosphors are demonstrated. The color conversion from blue to pure green is achieved by adding the
CsPbBr
3
-
OA
QDs solution up to 60 μL, while the pure green emission devices only need 18 μL
CsPbBr
3
-
DA
QDs solution under the same concentration. The ultrapure, highly efficient green light-emitting devices based on
CsPbBr
3
-
DA
QDs exhibit a luminous efficiency of 43.6 lm/W with a CIE (0.2086, 0.7635) under a 15.3 mA driving current. In addition, the green emission wavelength of the devices based on
CsPbBr
3
-
DA
QDs almost has no shift, even under a high injection current. These results highlight the promise of DA ligand-modified
CsPbBr
3
QDs for light-emitting devices and enrich the application field of ligand-modified
CsPbBr
3
QDs.
PDF全文
Full Text
Photonics Research
2020, 8(7): 07001086
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